Запис Детальніше

Incommensurate magnetism in the coupled spin tetrahedra system Cu₂Te₂O₅Cl₂

Vernadsky National Library of Ukraine

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Поле Співвідношення
 
Title Incommensurate magnetism in the coupled spin tetrahedra system Cu₂Te₂O₅Cl₂
 
Creator Zaharko, O.
Ronnow, H.M.
Daoud-Aladine, A.
Streule, S.
Juranyi, F.
Mesot, J.
Berger, H.
Brown, P.J.
 
Subject К семидесятилетию антиферромагнетизма
 
Description Neutron scattering studies on powder and single crystals have provided new evidences for unconventional
magnetism in Cu₂Te₂O₅Cl₂. The compound is built from tetrahedral clusters of S = 1/2
Cu²⁺ spins located on a tetragonal lattice. Magnetic ordering, emerging at TN = 18.2 K, leads to a
very complex multi-domain, most likely degenerate, ground state, which is characterized by an incommensurate
(ICM) wave vector k ~ [0.15, 0.42, 1/2]. The Cu²⁺ ions carry a magnetic moment
of 0.67(1) μB/Cu²⁺ at 1.5 K and form a four helices spin arrangement with two canted pairs
within the tetrahedra. A domain redistribution is observed when a magnetic field is applied in the
tetragonal plane (Hc ≈ 0.5 T), but not for H||c up to 4 T. The excitation spectrum is characterized
by two well-defined modes, one completely dispersionless at 6 meV, the other strongly dispersing
to a gap of 2 meV. The reason for such complex ground state and spin excitations may be geometrical
frustration of the Cu²⁺ spins within the tetrahedra, intra- and inter-tetrahedral couplings having
similar strengths and strong Dzyaloshinski–Moriya anisotropy. Candidates for the dominant
intra- and inter-tetrahedral interactions are proposed.
 
Date 2017-06-15T13:32:51Z
2017-06-15T13:32:51Z
2005
 
Type Article
 
Identifier Incommensurate magnetism in the coupled spin tetrahedra system Cu₂Te₂O₅Cl₂ / O. Zaharko, H.M. Ronnow, A. Daoud-Aladine, S. Streule, F. Juranyi, J. Mesot, H. Berger, P.J. Brown // Физика низких температур. — 2005. — Т. 31, № 8-9. — С. 1068-1072. — Бібліогр.: 17 назв. — англ.
0132-6414
PACS: 75.30.–m, 61.12.Ld, 75.10.Jm
http://dspace.nbuv.gov.ua/handle/123456789/121701
 
Language en
 
Relation Физика низких температур
 
Publisher Фізико-технічний інститут низьких температур ім. Б.І. Вєркіна НАН України