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Observation of the strain-driven charge-ordered state in La₀.₇Ca₀.₃MnO₃₋δ thin film with oxygen deficiency

Vernadsky National Library of Ukraine

Переглянути архів Інформація
 
 
Поле Співвідношення
 
Title Observation of the strain-driven charge-ordered state in La₀.₇Ca₀.₃MnO₃₋δ thin film with oxygen deficiency
 
Creator Prokhorov, V.G.
Komashko, V.A.
Kaminsky, G.G.
Svetchnikov, V.L.
Zandbergen, H.W.
Lee, Y.P.
Park, J.S.
Kim, K.W.
 
Subject Электpонные свойства металлов и сплавов
 
Description The magnetic and transport properties of La₀.₇Ca₀.₃MnO₃₋δ films with an oxygen deficiency (δ≃ 0.1) and a La₀.₉Ca₀.₁MnO₃ film with the stoichiometric oxygen content are investigated in a wide temperature range. It is shown that the charge-ordered insulating (COI) state is observed for a La₀.₇Ca₀.₃MnO₂.₉ film with thickness d ≤ 30 nm, which manifests mainly a cubic crystal structure with an anomalously small lattice parameter for this composition. An increase in the film thickness (d ≃ 60 nm) leads to a structural transition from the lattice-strained cubic to the relaxed rhombohedral phase, is accompanied by a shift of the Curie point (TC) to lower temperature and a frustration of the COI state. The magnetic and transport properties of the La₀.₇Ca₀.₃MnO₂.₉ film with d ≃ 60 nm are similar to those exhibited by the optimally oxygen-doped La₀.₉Ca₀.₁MnO₃ film. It is concluded that the formation of the COI state in the La₀.₇Ca₀.₃MnO₃₋δ compound is governed by a compression of the crystal lattice rather than accumulation of oxygen vacancies, the low doping of the substituted divalent ions, or electronic phase separation.
 
Date 2018-01-13T19:57:22Z
2018-01-13T19:57:22Z
2003
 
Type Article
 
Identifier Observation of the strain-driven charge-ordered state in La₀.₇Ca₀.₃MnO₃₋δ thin film with oxygen deficiency / V.G. Prokhorov, V.A. Komashko, G.G. Kaminsky, V.L. Svetchnikov, H.W. Zandbergen, Y.P. Lee, J.S. Park, K.W. Kim // Физика низких температур. — 2003. — Т. 29, № 2. — С. 161-168. — Бібліогр.: 23. назв. — англ.
0132-6414
PACS: 71.30.+h, 75.30.Vn, 75.70.-i
http://dspace.nbuv.gov.ua/handle/123456789/128785
 
Language en
 
Relation Физика низких температур
 
Publisher Фізико-технічний інститут низьких температур ім. Б.І. Вєркіна НАН України